POLYELECTROLYTES are water soluble polymer carrying ionic charge along the
polymer chain. Depending upon the charge, these polymers are anionic or
cationic. Polyelectrolytes are available in a wide range of molecular weights
and charge densities. Homo polymers of acrylamide are also included in the
family of polyelectrolytes though they do not carry any charge. These are called
nonionic. Polyelectrolytes have got a wide range of applications right from
water purification, oil recovery, colour removal, paper making, mineral
processing, etc., etc,. Polyelectrolytes are both flocculants as well as
deflocculants depending upon the molecular weight. A flocculant is
essentially a solid liquid separating agent while a deflocculant is a
dispersing agent.
HOW THE FLOCCULANTS WORK?
Stokes' Law
predicts that spherical particles suspended in a fluid medium settle at a rate
proportional to the fourth power of the particle radius. Thus large particles
will settle much faster than smaller ones. Most particles while suspended in
aqueous solution have a net negative surface charge.
This arises from
factors such as :
a) Unequal distribution of constituent ions on the particle
surface
b) Ionisation of surface groups pH effect
c) Specific
adsorption on the particle surface of ions from solution
d) Isomorphous
substitution of silicone atoms by aluminum atoms in an alumino silicate mineral
lattice (inorganic clays).
The above factors cause an electrical double layer
around each particle and colloidal particle in aqueous solution will not settle
very quickly. Interparticle interactions will cause repulsion and inspite
of Brownian motion trying to bring them together the suspension becomes stable,
i.e. the particles do not aggregate unless they are forced. The first phenomenon
taking place in the process of flocculation is the neutralisation of the nett
charge carried by each particle. Once charge neutralisation takes place several
particles come together which will result into coagulation. Flocculation is the
stage whereby the destabilised particles are induced to collect into larger
aggregates. The aggregation is followed by rapid settling as per Stokes' Law.
The various steps in the overall process are shown in Fig.1.
There are
two possible mechanisms given for the phenomena of polyelectrolyte induced
coagulation and flocculation. These are Charge patch model and Bridging model as
shown in Fig. 2 & 3. Polyelectrolyte flocculants can be generally divided
into two groups, depending on their molecular character and mode of
operation:
1) Primary coagulants (eg., polyamine types)
Have
high cationic charge density; satisfy the 'cationic demand' of the negatively
charged suspended particles and initiate coagulation and formation of
flocs.
Have low to medium molecular weight which allows a slow building of
flocs (provided there is an adequately long contact time between the forming
floc and the suspended matter) which gives a maximum removal of suspended solids
(maximum turbidity reduction).
2) Coagulation aids/flocculants (eg.,
polyacrylamides)
Have low charge density; are used only for building the
size of floc by bridging the primary flocs do not satisfy the 'charge
demand'.
Have very high molecular weight ; this is need to produce large,
fast settling flocs by bridging many small primary flocs.
The factors
affecting the selection of the appropriate polyelectrolyte(s) for a given
process are :
a) The nature of the suspended particles (substrate)
*
Organic/inorganic content
* Net surface charge density
* Solids content of
substrate
* pH of the substrate
* Temperature of the system (Brownian
motion).
b) The end result to be achieved
* Rapid separation of
the solid matter from the fluid
* Clarity of the separated fluid.
c)
Dynamic and shear effects
* Mixing /conditioning of polymer and
substrate
* Nature of the shear forces associated with the dewatering
equipment used.
TYPES OF POLYELECTROLYTES
Polyelectrolytes are
both inorganic and organic exhibiting both flocculation and deflocculation
properties. Inorganic polyelectrolytes exhibitingsedimentation properly are
coagulants rather than flocculants, whereas organic polyelectrolytes,
exhibiting sedimentation, property, are invariably high molecular weight
synthetic polymers. Inorganic flocculants are salts of multivalent metals like
aluminium and iron. The process of sedimentation these salts exhibit is totally
different from the organic types.
As discussed earlier depending on the
charge carried by the polymer, polyelectrolyte are classified into anionic
(negatively charged), cationic(positively charged) and nonionic (no charge). as
shown in Fig.4.
The acrylic acid unit of a polymer ionised to produce a
negatively charged polymer backbone. Since the charge carried by the active
portion of polymer is negative all such polyelectrolytes are known as anionics.
Similarly in the case of cationics the positive charge carrying nitrogen is a
part of the polymer. In the case of nonionics there is no charge on the base
polymer as there are no ionisable groups present in these.
The common anionic
polyelectrolytes are homo polymers and co polymers of NaSalt of acrylic acid
with acrylamide which are generally termed as polyacrylamides, eg :
Apart
from the above there are several other types of commercially available anionic
polyelectrolytes. The important ones are poly styrene sulfonic acids and
2acrylamido2methyl propane sulfonic acids. There are another series of
anionics which are derived from polyacrylamides by restricted hydrolysis to
produce anionic polyelectrolytes. These resemble copolymers of acrylamide and
acrylic acid.
Cationic polyelectrolytes are homopolymers or Copolymers
with Acrylamide of three major cationic monomers, viz. :
A wide range of
cationic polyelectrolytes are hence available depending on the cationic monomer
present, the charge density and the molecular weight.
Another less commonly
available cationic monomer is methacrylamido propyl trimethyl ammonium chloride
:
Quarternary polyamines which are manufactured from epichlorohydrine and a
secondary amine such as dimethylamine are another types of low molecular weight
cationics commonly found with very interesting applications.
Poly(dimethyl
diallyl ammoniam chloride) and copolymers with acrylamide are yet another type
of cationic. Polyethylene imines, which are cationics under acidic conditions,
are available as 2030% w/w aqueous solutions. These are generally highly
branched and are of low molecular weight in nature.
Similarly in the cationic
range, Mannich types are produced by reacting polyacrylamides with formaldehyde
and a secondary amine such as dimethyl amine and subsequently quarternising to
produce stable cationic polyelectrolytes.
The nonionic polyelectrolytes are
by and large homopolymers of acrylamide with a wide range of molecular weights.
Though countless polyelectrolytes are theoretically possible depending upon the
charge density and molecular weight a few of them have found commercial
application. This limits the usage of polyacrylamides of a specific pattern for
a specific application irrespective of the source of supply.
Methods
of Manufacturing
The conventional method of manufacturing
polyelectrolytes is by the solution polymerisation using a redox catalyst.
However, the viscosity of the polymer solution produced thus limits the
synthesis of high molecular weight polymers.
There are several polymers
available in the form of solutions of upto 50% concentration. As the ratio of
the acrylic acid to acrylamide goes up in an anionic polyelectrolyte the
viscosity built up is considerable which limits the practical use of this method
on an industrial scale.
Polyelectrolytes are also manufactured by the
emulsion polymerisation of acrylamide and a co monomer like acrylic acid or a
cationic monomer.
In this polymerisation process a stable water in oil
emulsion of the monomer is prepared and polymerised under conditions which are
much more isothermal using the oil phase to dissipate the heat of
polymerisation. The emulsion polymers have active polymer content generally
ranging from 25 to 50%. Certain additional surfactants are added to enable water
in oil emulsion to break and invert to oil in water emulsion at end users'
concentration. Wide ranging polyelectrolytes can be manufactured using this
emulsion polymerisation technique, however, the major disadvantages associated
could be :
i) Shelf life of the emulsions because emulsions are prone to
separate especially in high ambient temperatures, and
ii) When used in
application which require potable grade of polyelectrolytes because the oil used
for making emulsion cannot be removed prior to use.
Acrylamide has a very
fast propogation rate and a high exothermic heat of polymerisation. These
factors combine to give ato acceleration of polymerisation at high concentration
in aqueous solution with subsequent formation of a rubbery gel. The gel is,
subsequently granulated and then thermally dried to produce dry granular
polyelectrolytes.
DaiIchi Kogyo Seiyaku (DKS) has developed and
patented a continuous, photo initiated polymerisation process for manufacturing
the full range of Cationic, Anionic and Nonionic polyelectrolytes. In
collaboration with DKS, Dai Ichi Karkaria Ltd.,(DIKL) has set up s state of the
art plant to manufacture the full range of Polyelectrolyte in solid granular
form.
The salient features of the process are :
i) A monomer feed,
consisting of various types of monomers, initiators, chain terminators is first
made in a kettle.
ii) The above feed is photo polymerised in a specially
designed reactor to give a gel sheet.
iii) The gel sheet is further treated
to form uniform granules.
iv) Dehydration and blending of dry powders to
give a finished product and dry flowable granules.
The major advantages of
these processes are :
i) Very easy to manipulate the :
* Molecular weight,
from low to very high, by simply changing the feed composition
* The
composition of product by incorporating different monomers.
ii) Precise
control of charge density as the monomer feed composition is controlled at the
initial stages only.
iii) Precise control of molecular weight distribution
has the process in a continuous are :
a) No flammable and toxic solvents used
b) No production of waste matter or evolution of obnoxious gases
c) No
production of hazardous effluents.
The entire process is very clean and
apart from the above advantages, we can obtain product with very low residual
monomer contents, and hence can be used for potable applications also. The
finished products obtained are in the form of free flowing non dusting granules,
which possess a very long shelf life and are easy to sotre and handle.
By far
photo polymerisation has gained a prominent position in the industrial method of
manufacturing polyacrylamide type polyelectrolytes. The polymer produced is
having the same composition as the feed. Precise control of composition,
molecular weight and consistency of the product batch after batch are the
salient features of the process.
Polymers produced by the photo
polymerisation are by far the best type of polymers available in terms of its
high molecular weight though medium high molecular weight polymers can be made
by emulsion polymerisation technique though there are several draw backs
associated with this route. The first among these draw backs are the product
stability.
APPLICATION OF FLOCCULANTS
Major applications of
flocculants are their inherent solid liquid separating efficiency. This makes
polyelectrolytes a unique class of polymers which find extensive application in
potable water, industrial raw and process water, municipal sewage treatment,
mineral processing and metallurgy, oil drilling and recovery, paper and board
production, etc.
In all these applications the solid liquid separation
property is commercially exploited. The relation between the molecular size and
usage is summarised in Fig. 5
Flocculants also behave as filter aids by
modifying the filtration characteristics of suspended solids. Many of the
difficult to filter slurries are modified by the use of polymeric flocculants at
a relatively low dosage so that filtration rates become much faster. The ability
of flocculants to dewater slurry especially encountered in municipal sewage
treatment, mineral processing industry and metallurgical industry are tackled by
the use of high molecular weight flocculants.
Colour removal is another area
of application of flocculant. The charge carried by the polymer is responsible
for the abstraction of dissolved colouring matter from the waste water stream
and hence colour removing flocculants have wide applications in the waste water
treatment.
Removal of oil and grease especially from the waste water stream
is a second major application of speciality polymers. Low molecular weight
cationic polymers are extensively used for deoiling oil field effluents, waster
water coming out of refineries, engineering industries, etc.
Some of the
major areas of applications of polyelectrolytes are in the following
industries:
Potable water treatment
Drinking water is produced
by treating naturally occurring waters to reduce order, taste, appearance, and
sediment to acceptable levels. In general this involves removal of bacteria,
viruses, algae, dissolved mineral, dissolved organic matter and suspended solids
of the water. Flocculants are used to remove the latter two species. The
particle size and physical state are summarised in Fig.6 along with the
appropriate method generally adopted. Generally anionic polyacrylamide of low
degree of hydrolysis is used for the treatment of portable water. The polymers
used are governed by FDA standards that the residual acrylamide monomer content
in them be less than 0.05%. Since the turbidity in raw water is mainly due to
colloidal particles coagulation sedimentation and filtration are required. Hence
low molecular weight cationic flocculants are also popular for this
purpose.
Historically, inorganic coagulants based on Aluminium, Iron and
Calcium have been used for potable water treatment. Most common out of these is
aluminium sulphate (alum). These operate by formation of aluminium hydroxide
precipitate which sweeps down or coprecipitates the suspended matter. Apart
from the fact that these have to be used in large amounts, coagulants have
limited pH range under which hydroxide precipitates is formed.
This
increases the dissolved solids in the final drinking water, and may also cause
corrosion problems especially with Iron salts and generate excessive amounts of
sludges because of the voluminous nature of the metal hydroxide precipitates.
Polyelectrolytes can replace in part or whole, the inorganic coagulant to meet
the clarity norms at much reduced amounts (At ppm levels) and thereby
considerably reducing the sludge formation.
Waste water
treatment
Domestic and industrial effluents present a variety of
different types of the waste waters. Colour removal from the waste water stream
is a challenge to scientists o Water Chemistry. The colour, depending on the
source and nature can be removed by the following methods:
1) Chemical
destruction
2) Physical removal like adsorption
3) Physicochemical
methods
4) Biological methods.
Many of the colouring matters present in
the waste water stream can be reduced or oxidised. Oxidation method is preferred
when the colouring matter is of organic origin.
Sodium Hypochlorite, Hydrogen
Peroxide, etc. are commonly used for this purpose and the treatment is
expensive. Physical methods like adsorption has a limited application and
generally preferred in conjunction with other methods of treatment as a final
polishing step. Flocculant treatment may be called as physico chemical method as
both phenomena are involved in this process.
A typical example of this type
of product is DK SET CA 60. Treatment with DK SET CA 60 followed by DK SET P
3113 has been found to be an excellent combination for removing colour from
coloured waste water from Dyestuff Industries, textile mills, food processing
industries, distillery, pulp & paper, etc,. The cost of the treatment is
directly proportional to the intensity of the colouring
matter.
Municipal Sewage treatment
Municipal effluent is
treated in various ways depending on its composition, mainly to remove bioactive
materials from the produced water. Environmental issues have brought about
increasing pressure to remove all such materials including suspended solids from
sewage effluent. Polyelectrolytes can be used in some or all of the
sedimentation stages of the sewage treatment.
The main use of
polyelectrolytes as on date is for sludge dewatering. The optimum
polyelectrolyte molecular weight tend to increase depending on the type of
dewatering equipment used in the following order :
Drying bed << Vacuum
Filter
Belt Press < Filter Press < Centrifuge.
As the activated
sludge percentage goes up compared to the primary sludge requirement of polymer
is for a higher cationic charge. An increase in the proportion of activated
sludge to primary sludge decreases the overall dewaterability. At constant
molecular weight increasing the polymer cationic charge has very little effect
on the dewatering of primary sludge but improves the dewatering of 50:50 primary
: secondary sludge quite significantly.
Paper making
Paper making
is a very complex art. Apart from aiding paper mill effluent treatment,
polyelectrolytes have numerous applications in the actual manufacture of paper
and paper board:
a) Improving the retention on the paper machine of fibres,
fillers, dyestuffs and/or sizing chemicals
b) Improving paper machine
drainage (on machine dewatering)
c) Improving the 'dry strength' of paper
made with waste (recycled) fibres
d) Improvement of 'wet strength' of certain
paper grades such as facial tissues and kitchen towels.
Retention and
drainage are often parameters in opposition. Retention aids are generally
polyacrylamides anionic or cationic.
Dry strength resins improve the overall
strength of the finished paper by Hydrogen bonding between adjacent cellulose
fibres particles. These are generally low charge cationic polymers of moderate
molecular weight. Use of paper to abosrb moisture (facial tissue or kitchen
towels) require the paper to maintain its dimensional structure.
Mineral Processing
The mining and extraction of coal and
inorganic minerals from waste materials involves the use of large quantities of
water. Flocculants (invariably anionic polyacrylamides of high molecular weight)
are used to dewater the end product and/or the waste products ( tailings ) from
aqueous suspensions.
Very highly charged anionic polymers are used to settle
ion containing by products (red muds) in alumina production.
Oil field
applications
In contrast to the previously described application, areas
where the polyelectrolytes are generally employed for their flocculant ability,
the use of flocculant in the technology of drilling and exploration of oil
reserves from rock ormations also utilise the rheological properties of
polyelectrolyte in solutions. Almost all stages of the life cycle of an oil well
are potential application areas for polyelectrolytes. They find use during oil
(or gas) well drilling, well cementing, well reservoir stimulation, oil or gas
production, reservoir profile modification and enhanced oil recovery (Polymer
flooding).
Drilling muds
The proper functioning of a drilling
mud is very crucial to increase the drilling rate and efficiency of the drilling
operation without damaging the capacity of the well to yield oil. Polymers are
used to modify the mud viscosity as viscosifiers to increase the viscosity or as
low molecular weight thinners to decrease the viscosity of the mud under the
driling shear conditions.
Low to medium molecular weight polyacrylamides or
polyacrylates act as fluid loss additives to prevent synaeresis of mud or water
containing components of the mud into the reservoir formation which would block
the formation pores and limit egress during the production stage. Conversion of
high molecular weight anionic polyacrylamides are used to flocculate the spent
mud. Various polyelectrolytes can be used as friction reducers during the
fracturing process to stimulate the well.
Injection of suitably formulated
slugs of anionic polyacrylamide followed by dosing of multivalent metal ions
(particularly chromium) can produce in situ polymer cross linking which results
in a solid gel in the porous channels. Fluid flow is therefore diverted to
narrower channels since the fluid cannot penetrate the gel. This phenomenon is
known as profile modification.
Enhanced oil recovery also known as improved
oil recovery employs techniques to extract more oil. High molecular weight
polyacrylamides in dilute solution increase the viscosity of water above that of
oil. Polymer flooding involves injection of polyacrylamide solution into the
well to displace the oil which is of lower viscosity.
POLYELECTROLYTES AS ANTISCALANTS AND DISPERSANTS
Antiscalants
either prevent scale formation entirely or permit the scale only to be deposited
in such a way that it is easily removed by the fluid flowing along the pipe or
heat transfer surface. Dispersants do not stop the formation of scale, but are
able to keep the scale particles in suspension in the bulk fluid. Chemically
antiscalants and dispersants are low molecular weight anionic polyelectrolytes,
being polymers of acrylic acid and its salts, copolymers of acrylamide and
acrylic acid. Molecular weights vary in the range of 1000 to 100000 with anti
scalants being at the lower end of the range and dispersants, eg., polymers used
in laundry detergent formulations at the upper end.
Proper selection of
polymer composition molecular weight and molecular weight distribution makes
these products excellent for uses in :
1) Boiler treatment
2) Cooling
towers and air conditioning systems
3) Desalination of water (brackish or sea
water) by either
a) High temperature evaporative processes, such as
MultiStage Flash(MSF) Evaporation
b) Ambient temperature processes, such
as Reverse Osmosis(RO).
4) Sugar production
5) Mineral processing
(kaolinite, calcium carbonate)
6) Papermaking (dispersants for the above
minerals used as paper fillers)
7) Oil Drilling mud dispersants ('mud
thinners')
8) Oil production.
(DK SET is the brand name of polyacrylamides
manufactured by DaiIchi Karkaria Ltd., using the Photopolymerization
Technology of DaiIchi Kogyo Seiyaku Co.,
Japan.)
bibliography
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volumes),1984.
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36043R1 Ohio, USA, 1988.
* Hoover, M.F., Cationic quarternary
polyelectrolytesA literature review J. Macromol,
Sci.Chem.,A4(1970)1327.
* Halverson,F&Panzer, H.P.Flocculating
agents. In Encyclopedia of Chemical Technology, Volume10,3rd Edition,
ed.R.E.Kirk and D.
* DaiIchi Karkaria Ltd. Product brochure of DK SET
flocculants.
* Bikales M.M.,Water Soluble Polymers, Plenum Press, NY 1973.